RESUMEN
We report a single-photon Mach-Zehnder interferometer stabilized to a phase precision of 0.05 degrees over 15 hours. To lock the phase, we employ an auxiliary reference light at a different wavelength than the quantum signal. The developed phase locking operates continuously, with negligible crosstalk, and for an arbitrary phase of the quantum signal. Moreover, its performance is independent of intensity fluctuations of the reference. Since the presented method can be used in a vast majority of quantum interferometric networks it can significantly improve phase-sensitive applications in quantum communication and quantum metrology.
RESUMEN
We report a non-blocking high-resolution digital delay line based on an asynchronous circuit design. Field-programmable gate array logic primitives were used as a source of delay and optimally arranged using combinatorial optimization. This approach allows for an efficient trade-off of the resolution and a delay range together with a minimized dead time operation. We demonstrate the method by implementing the delay line adjustable from 23 ns up to 1635 ns with a resolution of 10 ps. We present a detailed experimental characterization of the device focusing on thermal instability, timing jitter, and pulse spreading, which represent three main issues of the asynchronous design. We found a linear dependence of the delay on the temperature with the slope of 0.2 ps K-1 per logic primitive. We measured the timing jitter of the delay to be in the range of 7-165 ps, linearly increasing over the dynamic range of the delay. We reduced the effect of pulse spreading by introducing pulse shrinking circuits and reached the overall dead time of 4-22.5 ns within the dynamic range of the delay. The presented non-blocking delay line finds usage in applications where the dead time minimization is crucial, and tens of picoseconds of excess jitter is acceptable, such as in many advanced photonic networks.
RESUMEN
We report a measurement workflow free of systematic errors consisting of a reconfigurable photon-number-resolving detector, custom electronic circuitry, and faithful data-processing algorithm. We achieve an unprecedented accurate measurement of various photon-number distributions going beyond the number of detection channels with an average fidelity of 0.998, where the error is primarily caused by the sources themselves. Mean numbers of photons cover values up to 20 and faithful autocorrelation measurements range from g^{(2)}=6×10^{-3} to 2. We successfully detect chaotic, classical, nonclassical, non-Gaussian, and negative-Wigner-function light. Our results open new paths for optical technologies by providing full access to the photon-number information without the necessity of detector tomography.
RESUMEN
Spectroscopy of vibrational optical activity has been established as a powerful tool to study molecular structures and interactions. In most cases, only fundamental molecular transitions are analyzed. In the present study, we analyze a broader range of vibrational frequencies (40-4000 cm-1), which could be measured on a new Raman optical activity (ROA) instrument. An unexpectedly strong vibrational Raman optical activity of 2-chloropropionitrile has been observed within the low-frequency region (40-150 cm-1). On the basis of combined molecular dynamics and density functional theory simulations, it could be assigned to intermolecular vibrations. A detailed analysis also revealed connection between spectral shapes and molecular structure and flexibility, such as bending of the CCN group. At the other edge of the scale, within â¼1500-4000 cm-1, for the first time, many combination and overtone ROA bands have been observed for 2-chloropropionitrile and α-pinene. These were also partially assigned, using quantum-chemical computations. The band assignment was confirmed by a comparison with Raman, absorption, and vibrational circular dichroism spectra. The measurement in the broader vibrational range thus significantly extends the information that can be obtained by optical spectroscopy, including intermolecular interactions of chiral molecules and liquids.