Your browser doesn't support javascript.
loading
Mostrar: 20 | 50 | 100
Resultados 1 - 20 de 33
Filtrar
Más filtros











Base de datos
Intervalo de año de publicación
1.
Phys Rev E ; 110(2-1): 024143, 2024 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-39295067

RESUMEN

We study analytically the ordering kinetics and the final metastable states in the three-dimensional long-range voter model where N agents described by a Boolean spin variable S_{i} can be found in two states (or opinion) ±1. The kinetics is such that each agent copies the opinion of another at distance r chosen with probability P(r)∝r^{-α} (α>0). In the thermodynamic limit N→∞ the system approaches a correlated metastable state without consensus, namely without full spin alignment. In such states the equal-time correlation function C(r)=〈S_{i}S_{j}〉 (where r is the i-j distance) decreases algebraically in a slow, nonintegrable way. Specifically, we find C(r)∼r^{-1}, or C(r)∼r^{-(6-α)}, or C(r)∼r^{-α} for α>5, 3<α≤5, and 0≤α≤3, respectively. In a finite system metastability is escaped after a time of order N and full ordering is eventually achieved. The dynamics leading to metastability is of the coarsening type, with an ever-increasing correlation length L(t) (for N→∞). We find L(t)∼t^{1/2} for α>5, L(t)∼t^{5/2α} for 4<α≤5, and L(t)∼t^{5/8} for 3≤α≤4. For 0≤α<3 there is not macroscopic coarsening because stationarity is reached in a microscopic time. Such results allow us to conjecture the behavior of the model for generic spatial dimension.

2.
Phys Rev E ; 109(3-1): 034133, 2024 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-38632821

RESUMEN

We study analytically the ordering kinetics of the two-dimensional long-range voter model on a two-dimensional lattice, where agents on each vertex take the opinion of others at distance r with probability P(r)∝r^{-α}. The model is characterized by different regimes, as α is varied. For α>4, the behavior is similar to that of the nearest-neighbor model, with the formation of ordered domains of a typical size growing as L(t)∝sqrt[t], until consensus is reached in a time of the order of NlnN, with N being the number of agents. Dynamical scaling is violated due to an excess of interfacial sites whose density decays as slowly as ρ(t)∝1/lnt. Sizable finite-time corrections are also present, which are absent in the case of nearest-neighbor interactions. For 0<α≤4, standard scaling is reinstated and the correlation length increases algebraically as L(t)∝t^{1/z}, with 1/z=2/α for 3<α<4 and 1/z=2/3 for 0<α<3. In addition, for α≤3, L(t) depends on N at any time t>0. Such coarsening, however, only leads the system to a partially ordered metastable state where correlations decay algebraically with distance, and whose lifetime diverges in the N→∞ limit. In finite systems, consensus is reached in a time of the order of N for any α<4.

3.
Phys Rev E ; 108(4-1): 044131, 2023 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-37978597

RESUMEN

We investigate the influence of long-range (LR) interactions on the phase ordering dynamics of the one-dimensional random-field Ising model (RFIM). Unlike the usual RFIM, a spin interacts with all other spins through a ferromagnetic coupling that decays as r^{-(1+σ)}, where r is the distance between two spins. In the absence of LR interactions, the size of coarsening domains R(t) exhibits a crossover from pure system behavior R(t)∼t^{1/2} to an asymptotic regime characterized by logarithmic growth: R(t)∼(lnt)^{2}. The LR interactions affect the preasymptotic regime, which now exhibits ballistic growth R(t)∼t, followed by σ-dependent growth R(t)∼t^{1/(1+σ)}. Additionally, the LR interactions also affect the asymptotic logarithmic growth, which becomes R(t)∼(lnt)^{α(σ)} with α(σ)<2. Thus, LR interactions lead to faster growth than for the nearest-neighbor system at short times. Unexpectedly, this driving force causes a slowing down of the dynamics (α<2) in the asymptotic logarithmic regime. This is explained in terms of a nontrivial competition between the pinning force caused by the random field and the driving force introduced by LR interactions. We also study the spatial correlation function and the autocorrelation function of the magnetization field. The former exhibits superuniversality for all σ, i.e., a scaling function that is independent of the disorder strength. The same holds for the autocorrelation function when σ<1, whereas a signature of the violation of superuniversality is seen for σ>1.

4.
Adv Mater ; 35(15): e2211157, 2023 Apr.
Artículo en Inglés | MEDLINE | ID: mdl-36648210

RESUMEN

Device performance of solution-processed 2D semiconductors in printed electronics has been limited so far by structural defects and high interflake junction resistance. Covalently interconnected networks of transition metal dichalcogenides potentially represent an efficient strategy to overcome both limitations simultaneously. Yet, the charge-transport properties in such systems have not been systematically researched. Here, the charge-transport mechanisms of printed devices based on covalent MoS2 networks are unveiled via multiscale analysis, comparing the effects of aromatic versus aliphatic dithiolated linkers. Temperature-dependent electrical measurements reveal hopping as the dominant transport mechanism: aliphatic systems lead to 3D variable range hopping, unlike the nearest neighbor hopping observed for aromatic linkers. The novel analysis based on percolation theory attributes the superior performance of devices functionalized with π-conjugated molecules to the improved interflake electronic connectivity and formation of additional percolation paths, as further corroborated by density functional calculations. Valuable guidelines for harnessing the charge-transport properties in MoS2 devices based on covalent networks are provided.

5.
Phys Rev E ; 105(3-1): 034131, 2022 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-35428063

RESUMEN

It is known that, after a quench to zero temperature (T=0), two-dimensional (d=2) Ising ferromagnets with short-range interactions do not always relax to the ordered state. They can also fall in infinitely long-lived striped metastable states with a finite probability. In this paper, we study how the abundance of striped states is affected by long-range interactions. We investigate the relaxation of d=2 Ising ferromagnets with power-law interactions by means of Monte Carlo simulations at both T=0 and T≠0. For T=0 and the finite system size, the striped metastable states are suppressed by long-range interactions. In the thermodynamic limit, their occurrence probabilities are consistent with the short-range case. For T≠0, the final state is always ordered. Further, the equilibration occurs at earlier times with an increase in the strength of the interactions.

6.
Phys Rev Lett ; 127(12): 128301, 2021 Sep 17.
Artículo en Inglés | MEDLINE | ID: mdl-34597111

RESUMEN

Zipf's law describes the empirical size distribution of the components of many systems in natural and social sciences and humanities. We show, by solving a statistical model, that Zipf's law co-occurs with the maximization of the diversity of the component sizes. The law ruling the increase of such diversity with the total dimension of the system is derived and its relation with Heaps's law is discussed. As an example, we show that our analytical results compare very well with linguistics and population datasets.

7.
Phys Rev E ; 103(1-1): 012108, 2021 Jan.
Artículo en Inglés | MEDLINE | ID: mdl-33601633

RESUMEN

We study the low-temperature domain growth kinetics of the two-dimensional Ising model with long-range coupling J(r)∼r^{-(d+σ)}, where d=2 is the dimensionality. According to the Bray-Rutenberg predictions, the exponent σ controls the algebraic growth in time of the characteristic domain size L(t), L(t)∼t^{1/z}, with growth exponent z=1+σ for σ<1 and z=2 for σ>1. These results hold for quenches to a nonzero temperature T>0 below the critical temperature T_{c}. We show that, in the case of quenches to T=0, due to the long-range interactions, the interfaces experience a drift which makes the dynamics of the system peculiar. More precisely, we find that in this case the growth exponent takes the value z=4/3, independently of σ, showing that it is a universal quantity. We support our claim by means of extended Monte Carlo simulations and analytical arguments for single domains.

8.
Phys Rev E ; 102(2-1): 020102, 2020 Aug.
Artículo en Inglés | MEDLINE | ID: mdl-32942398

RESUMEN

We discuss the interplay between the degree of dynamical stochasticity, memory persistence, and violation of the self-averaging property in the aging kinetics of quenched ferromagnets. We show that, in general, the longest possible memory effects, which correspond to the slowest possible temporal decay of the correlation function, are accompanied by the largest possible violation of self-averaging and a quasideterministic descent into the ergodic components. This phenomenon is observed in different systems, such as the Ising model with long-range interactions, including the mean-field, and the short-range random-field Ising model.

9.
Biophys J ; 119(4): 873-883, 2020 08 18.
Artículo en Inglés | MEDLINE | ID: mdl-32738219

RESUMEN

The phase separation occurring in a system of mutually interacting proteins that can bind on specific sites of a chromatin fiber is investigated here. This is achieved by means of extensive molecular dynamics simulations of a simple polymer model that includes regulatory proteins as interacting spherical particles. Our interest is particularly focused on the role played by phase separation in the formation of molecule aggregates that can join distant regulatory elements, such as gene promoters and enhancers, along the DNA. We find that the overall equilibrium state of the system resulting from the mutual interplay between binding molecules and chromatin can lead, under suitable conditions that depend on molecules concentration, molecule-molecule, and molecule-DNA interactions, to the formation of phase-separated molecular clusters, allowing robust contacts between regulatory sites. Vice versa, the presence of regulatory sites can promote the phase-separation process. Different dynamical regimes can generate the enhancer-promoter contact, either by cluster nucleation at binding sites or by bulk spontaneous formation of the mediating cluster to which binding sites are successively attracted. The possibility that such processes can explain experimental live-cell imaging data measuring distances between regulatory sites during time is also discussed.


Asunto(s)
Cromatina , Elementos de Facilitación Genéticos , Comunicación , Modelos Químicos , Modelos Genéticos , Simulación de Dinámica Molecular , Regiones Promotoras Genéticas
10.
Phys Rev E ; 99(1-1): 012131, 2019 Jan.
Artículo en Inglés | MEDLINE | ID: mdl-30780308

RESUMEN

We study numerically the aging properties of the two-dimensional Ising model with quenched disorder considered in our recent paper [Phys. Rev. E 95, 062136 (2017)2470-004510.1103/PhysRevE.95.062136], where frustration can be tuned by varying the fraction of antiferromagnetic interactions. Specifically, we focus on the scaling properties of the autocorrelation and linear response functions after a quench of the model to a low temperature. We find that the interplay between equilibrium and aging occurs differently in the various regions of the phase diagram of the model. When the quench is made into the ferromagnetic phase the two-time quantities are made by the sum of an equilibrium and an aging part, whereas in the paramagnetic phase these parts combine in a multiplicative way. Scaling forms are shown to be obeyed with good accuracy, and the corresponding exponents and scaling functions are determined and discussed in the framework of what is known in clean and disordered systems.

11.
Entropy (Basel) ; 21(3)2019 Mar 21.
Artículo en Inglés | MEDLINE | ID: mdl-33267026

RESUMEN

In this paper we review some general properties of probability distributions which exhibit a singular behavior. After introducing the matter with several examples based on various models of statistical mechanics, we discuss, with the help of such paradigms, the underlying mathematical mechanism producing the singularity and other topics such as the condensation of fluctuations, the relationships with ordinary phase-transitions, the giant response associated to anomalous fluctuations, and the interplay with fluctuation relations.

12.
Phys Rev E ; 95(6-1): 062136, 2017 Jun.
Artículo en Inglés | MEDLINE | ID: mdl-28709286

RESUMEN

We study numerically a two-dimensional random-bond Ising model where frustration can be tuned by varying the fraction a of antiferromagnetic coupling constants. At low temperatures the model exhibits a phase with ferromagnetic order for sufficiently small values of a, aa_{a}, an antiferromagnetic phase exists. After a deep quench from high temperatures, slow evolution is observed for any value of a. We show that different amounts of frustration, tuned by a, affect the dynamical properties in a highly nontrivial way. In particular, the kinetics is logarithmically slow in phases with ferromagnetic or antiferromagnetic order, whereas evolution is faster, i.e., algebraic, when spin-glass order is prevailing. An interpretation is given in terms of the different nature of phase space.

13.
Phys Rev E ; 95(3-1): 032136, 2017 Mar.
Artículo en Inglés | MEDLINE | ID: mdl-28415228

RESUMEN

We study the evolution leading to (or regressing from) a large fluctuation in a statistical mechanical system. We introduce and study analytically a simple model of many identically and independently distributed microscopic variables n_{m} (m=1,M) evolving by means of a master equation. We show that the process producing a nontypical fluctuation with a value of N=∑_{m=1}^{M}n_{m} well above the average 〈N〉 is slow. Such process is characterized by the power-law growth of the largest possible observable value of N at a given time t. We find similar features also for the reverse process of the regression from a rare state with N≫〈N〉 to a typical one with N≃〈N〉.

14.
Phys Rev E ; 95(2-1): 022101, 2017 Feb.
Artículo en Inglés | MEDLINE | ID: mdl-28297910

RESUMEN

By studying numerically the phase-ordering kinetics of a two-dimensional ferromagnetic Ising model with quenched disorder (either random bonds or random fields) we show that a critical percolation structure forms at an early stage. This structure is then rendered more and more compact by the ensuing coarsening process. Our results are compared to the nondisordered case, where a similar phenomenon is observed, and they are interpreted within a dynamical scaling framework.

15.
Phys Rev E ; 93(5): 052105, 2016 05.
Artículo en Inglés | MEDLINE | ID: mdl-27300828

RESUMEN

We study numerically the two-dimensional Ising model with nonconserved dynamics quenched from an initial equilibrium state at the temperature T_{i}≥T_{c} to a final temperature T_{f} below the critical one. By considering processes initiating both from a disordered state at infinite temperature T_{i}=∞ and from the critical configurations at T_{i}=T_{c} and spanning the range of final temperatures T_{f}∈[0,T_{c}[ we elucidate the role played by T_{i} and T_{f} on the aging properties and, in particular, on the behavior of the autocorrelation C and of the integrated response function χ. Our results show that for any choice of T_{f}, while the autocorrelation function exponent λ_{C} takes a markedly different value for T_{i}=∞ [λ_{C}(T_{i}=∞)≃5/4] or T_{i}=T_{c} [λ_{C}(T_{i}=T_{c})≃1/8] the response function exponents are unchanged. Supported by the outcome of the analytical solution of the solvable spherical model we interpret this fact as due to the different contributions provided to autocorrelation and response by the large-scale properties of the system. As changing T_{f} is considered, although this is expected to play no role in the large-scale and long-time properties of the system, we show important effects on the quantitative behavior of χ. In particular, data for quenches to T_{f}=0 are consistent with a value of the response function exponent λ_{χ}=1/2λ_{C}(T_{i}=∞)=5/8 different from the one [λ_{χ}∈(0.5-0.56)] found in a wealth of previous numerical determinations in quenches to finite final temperatures. This is interpreted as due to important preasymptotic corrections associated to T_{f}>0.

16.
Artículo en Inglés | MEDLINE | ID: mdl-26172676

RESUMEN

We study numerically the coarsening dynamics of the Ising model on a regular lattice with random bonds and on deterministic fractal substrates. We propose a unifying interpretation of the phase-ordering processes based on two classes of dynamical behaviors characterized by different growth laws of the ordered domain size, namely logarithmic or power law, respectively. It is conjectured that the interplay between these dynamical classes is regulated by the same topological feature that governs the presence or the absence of a finite-temperature phase transition.

17.
Artículo en Inglés | MEDLINE | ID: mdl-25122287

RESUMEN

Condensation of fluctuations is an interesting phenomenon conceptually distinct from condensation on average. One striking feature is that, contrary to what happens on average, condensation of fluctuations may occur even in the absence of interaction. The explanation emerges from the duality between large deviation events in the given system and typical events in a new and appropriately biased system. This phenomenon is investigated in the context of the Gaussian model, chosen as a paradigmatical noninteracting system, before and after an instantaneous temperature quench. It is shown that the bias induces a mean-field-like effective interaction responsible for the condensation on average. Phase diagrams, covering both the equilibrium and the off-equilibrium regimes, are derived for observables representative of generic behaviors.


Asunto(s)
Modelos Teóricos , Transición de Fase , Distribución Normal , Termodinámica
18.
Artículo en Inglés | MEDLINE | ID: mdl-24229138

RESUMEN

We study numerically the phase-ordering kinetics of the two-dimensional site-diluted Ising model. The data can be interpreted in a framework motivated by renormalization-group concepts. Apart from the usual fixed point of the nondiluted system, there exist two disorder fixed points, characterized by logarithmic and power-law growth of the ordered domains. This structure gives rise to a rich scaling behavior, with an interesting crossover due to the competition between fixed points, and violation of superuniversality.

19.
Phys Rev E Stat Nonlin Soft Matter Phys ; 86(6 Pt 1): 061129, 2012 Dec.
Artículo en Inglés | MEDLINE | ID: mdl-23367915

RESUMEN

We use state-of-the-art molecular dynamics simulations to study hydrodynamic effects on aging during kinetics of phase separation in a fluid mixture. The domain growth law shows a crossover from a diffusive regime to a viscous hydrodynamic regime. There is a corresponding crossover in the autocorrelation function from a power-law behavior to an exponential decay. While the former is consistent with theories for diffusive domain growth, the latter results as a consequence of faster advective transport in fluids for which an analytical justification has been provided.

20.
Phys Rev E Stat Nonlin Soft Matter Phys ; 81(1 Pt 1): 011124, 2010 Jan.
Artículo en Inglés | MEDLINE | ID: mdl-20365340

RESUMEN

We discuss the relation between the fluctuation-dissipation relation derived by Chatelain and Ricci-Tersenghi [C. Chatelain, J. Phys. A 36, 10739 (2003); F. Ricci-Tersenghi, Phys. Rev. E 68, 065104(R) (2003)] and that by Lippiello-Corberi-Zannetti [E. Lippiello, F. Corberi, and M. Zannetti, Phys. Rev. E 71, 036104 (2005)]. In order to do that, we rederive the fluctuation-dissipation relation for systems of discrete variables evolving in discrete time via a stochastic nonequilibrium Markov process. The calculation is carried out in a general formalism comprising the Chatelain, Ricci-Tersenghi, result and that by Lippiello-Corberi-Zannetti as special cases. The applicability, generality, and experimental feasibility of the two approaches are thoroughly discussed. Extending the analytical calculation to the variance of the response function, we show the advantage of field-free numerical methods with respect to the standard method, where the perturbation is applied. We also show that the signal-to-noise ratio is better (by a factor square root of 2) in the algorithm of Lippiello-Corberi-Zannetti with respect to that of Chatelain-Ricci Tersenghi.

SELECCIÓN DE REFERENCIAS
DETALLE DE LA BÚSQUEDA