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1.
Nano Lett ; 20(7): 5408-5414, 2020 Jul 08.
Artículo en Inglés | MEDLINE | ID: mdl-32470310

RESUMEN

Graphene quantum dots (GQDs) have recently attracted considerable attention, with appealing properties for terahertz (THz) technology. This includes the demonstration of large thermal bolometric effects in GQDs when illuminated by THz radiation. However, the interaction of THz photons with GQDs in the Coulomb blockade regime, i.e., single electron transport regime, remains unexplored. Here, we demonstrate the ultrasensitive photoresponse to THz radiation (from <0.1 to 10 THz) of a hBN-encapsulated GQD in the Coulomb blockade regime at low temperature (170 mK). We show that THz radiation of ∼10 pW provides a photocurrent response in the nanoampere range, resulting from a renormalization of the chemical potential of the GQD of ∼0.15 meV. We attribute this photoresponse to an interfacial photogating effect. Furthermore, our analysis reveals the absence of thermal effects, opening new directions in the study of coherent quantum effects at THz frequencies in GQDs.

2.
Phys Rev Lett ; 122(16): 165301, 2019 Apr 26.
Artículo en Inglés | MEDLINE | ID: mdl-31075030

RESUMEN

Helium is recognized as a model system for the study of phase transitions. Of particular interest is the superfluid phase in two dimensions. We report measurements on superfluid helium films adsorbed on the surface of a suspended carbon nanotube. We measure the mechanical vibrations of the nanotube to probe the adsorbed helium film. We demonstrate the formation of helium layers up to five atoms thickness. Upon increasing the vapor pressure, we observe layer-by-layer growth with discontinuities in both the number of adsorbed atoms and the speed of the third sound in the adsorbed film. These hitherto unobserved discontinuities point to a series of first-order layering transitions. Our results show that helium multilayers adsorbed on a nanotube are of unprecedented quality compared to previous works. They pave the way to new studies of quantized superfluid vortex dynamics on cylindrical surfaces, of the Berezinskii-Kosterlitz-Thouless phase transition in this new geometry, and perhaps also to supersolidity in crystalline single layers as predicted in quantum Monte Carlo calculations.

3.
Phys Rev Lett ; 114(16): 165301, 2015 Apr 24.
Artículo en Inglés | MEDLINE | ID: mdl-25955054

RESUMEN

We report the results of flow experiments in which two chambers containing solid ^{4}He are connected by a superfluid Vycor channel. At low temperatures and pressures, mechanically squeezing the solid in one chamber produced a pressure increase in the second chamber, a measure of mass transport through our solid-superfluid-solid junction. This pressure response is very similar to the flow seen in recent experiments at the University of Massachusetts: it began around 600 mK, increased as the temperature was reduced, then decreased dramatically at a temperature, T_{d}, which depended on the ^{3}He impurity concentration. Our experiments indicate that the flow is limited by mass transfer across the solid-liquid interface near the Vycor ends, where the ^{3}He collects at low temperature, rather than by flow paths within the solid ^{4}He.

4.
Phys Rev Lett ; 111(11): 119602, 2013 Sep 13.
Artículo en Inglés | MEDLINE | ID: mdl-24074125
5.
Phys Rev Lett ; 110(3): 035301, 2013 Jan 18.
Artículo en Inglés | MEDLINE | ID: mdl-23373930

RESUMEN

When submitted to large stresses at high temperature, usual crystals may irreversibly deform. This phenomenon is known as plasticity and it is due to the motion of crystal defects such as dislocations. We have discovered that, in the absence of impurities and in the zero temperature limit, helium 4 crystals present a giant plasticity that is anisotropic and reversible. Direct measurements on oriented single crystals show that their resistance to shear nearly vanishes in one particular direction because dislocations glide freely parallel to the basal planes of the hexagonal structure. This plasticity disappears as soon as traces of helium 3 impurities bind to the dislocations or if their motion is damped by collisions with thermal phonons.

6.
J Chem Phys ; 133(17): 174507, 2010 Nov 07.
Artículo en Inglés | MEDLINE | ID: mdl-21054051

RESUMEN

We report on the simultaneous measurements of the speed of sound and the density in liquid water under negative pressure. Application of a focused acoustic wave to the bulk liquid is able to generate negative pressures before nucleation of the vapor phase occurs. A method for time-resolved Brillouin scattering is developed to measure the speed of sound during the passage of a 1 MHz ultrasonic wave. This is coupled with a fiber optic probe hydrophone which allows the determination of the density. Together, these methods give an ambient temperature equation of state of metastable liquid water down to the acoustic cavitation threshold. Empirical equations of state of water are based on experimental data at positive pressure; the validity of their extrapolation to negative pressures had been tested only indirectly or with very weakly metastable liquid. We provide thermodynamic data that prove the fidelity of recent equations of state down to -26 MPa. However, this raises questions regarding the nature of the cavitation threshold observed in acoustic experiments, which is far less negative than expected.

7.
Nature ; 464(7286): 176-82, 2010 Mar 11.
Artículo en Inglés | MEDLINE | ID: mdl-20220834

RESUMEN

A 'supersolid' is a quantum solid in which a fraction of the mass is superfluid. As a remarkable consequence, it is rigid, but part of its mass is able to flow owing to quantum physical processes. This paradoxical state of matter was considered as a theoretical possibility as early as 1969, but its existence was discovered only in 2004, in (4)He. Since then, intense experimental and theoretical efforts have been made to explain the origins of this exotic state of matter. It now seems that its physical interpretation is more complicated than originally thought.

8.
Phys Rev Lett ; 105(14): 145302, 2010 Oct 01.
Artículo en Inglés | MEDLINE | ID: mdl-21230841

RESUMEN

We have measured the elasticity of high quality ultrapure 4He single crystals in the low temperature region where supersolidity is supposed to occur. At 20 mK, our results are consistent with elastic coefficients previously measured at 1.2 K. As the temperature increases from 20 to 100 mK, a large softening occurs because dislocations unpin from ³He impurities. In the absence of ³He impurities, dislocations are free to move down to 20 mK; the crystals are soft. The large magnitude of this anomalous softening shows that dislocations form a mobile mosaic structure. It illustrates the remarkable quantum plasticity of 4He crystals.

9.
Phys Rev Lett ; 101(18): 189601; author reply 189602, 2008 Oct 31.
Artículo en Inglés | MEDLINE | ID: mdl-18999871
10.
Nature ; 451(7175): 136-7, 2008 Jan 10.
Artículo en Inglés | MEDLINE | ID: mdl-18185577
11.
Phys Rev Lett ; 99(20): 205302, 2007 Nov 16.
Artículo en Inglés | MEDLINE | ID: mdl-18233154

RESUMEN

We have observed boundaries between hcp 4He crystal grains in equilibrium with liquid 4He. We have found that, when emerging at the liquid-solid interface, a grain boundary makes a groove whose dihedral angle 2theta is nonzero. This measurement shows that grain boundaries are not completely wet by the liquid phase, in agreement with recent Monte Carlo simulations. Depending on the value of theta, the contact line of a grain boundary with a solid wall may be wet by the liquid. In this case, the line is a thin channel with a curved triangular cross section, whose measured width agrees with predictions from a simple model. We discuss these measurements in the context of grain boundary premelting and for a future understanding of the possible supersolidity of solid 4He.

12.
Phys Rev E Stat Nonlin Soft Matter Phys ; 74(4 Pt 1): 041603, 2006 Oct.
Artículo en Inglés | MEDLINE | ID: mdl-17155066

RESUMEN

We investigate the limiting mechanical tension (negative pressure) that liquid water can sustain before cavitation occurs. The temperature dependence of this quantity is of special interest for water, where it can be used as a probe of a postulated anomaly of its equation of state. After a brief review of previous experiments on cavitation, we describe our method which consists in focusing a high amplitude sound wave in the bulk liquid, away from any walls. We obtain highly reproducible results, allowing us to study in detail the statistics of cavitation, and to give an accurate definition of the cavitation threshold. Two independent pressure calibrations are performed. The cavitation pressure is found to increase monotonically from -26 MPa at 0 degrees C to -17 MPa at 80 degrees C. While these values lie among the most negative pressures reported in water, they are still far away from the cavitation pressure expected theoretically and reached in the experiment by Angell and his group [Zheng, Science 254, 829 (1991)] (around -120 MPa at 40 degrees C). Possible reasons for this discrepancy are considered.

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